Second-harmonic generation and reflecance-anisotropy spectroscopy of vicinal Si(001)

dc.contributor.advisorDowner, Michael Coffinen
dc.creatorKwon, Jinheeen
dc.date.accessioned2008-08-28T23:06:39Zen
dc.date.available2008-08-28T23:06:39Zen
dc.date.issued2006en
dc.descriptiontexten
dc.description.abstractSpectroscopic second-harmonic generation (SHG) and reflectance-anisotropy spectroscopy (RAS) of native-oxidized vicinal Si(001) with off-cut angles ζ = 0o , 4o , 6o , 8o and 10o from (001) toward [110] are performed. The SHG spectra are first decomposed using the macroscopic Fourier analysis. As a common microscopic analysis for SHG and RAS, we use a simplified bond hyperpolarizability model. The description of the expanded bond model and the result of the calculation are presented. The derived complex hyperpolarizability spectra are compared with the corresponding inverted real and imaginary parts using nonlinear Kramers-Kronig relations, thus confirming the consistency of the developed bond model. RAS and SHG spectra from clean and selectively H2 adsorbed reconstructed vicinal Si(001):6o surfaces are obtained and analyzed in a similar way.
dc.description.departmentPhysicsen
dc.format.mediumelectronicen
dc.identifierb65464242en
dc.identifier.oclc156471145en
dc.identifier.urihttp://hdl.handle.net/2152/2750en
dc.language.isoengen
dc.rightsCopyright is held by the author. Presentation of this material on the Libraries' web site by University Libraries, The University of Texas at Austin was made possible under a limited license grant from the author who has retained all copyrights in the works.en
dc.subject.lcshSecond harmonic generationen
dc.subject.lcshAnisotropyen
dc.subject.lcshSpectrum analysisen
dc.titleSecond-harmonic generation and reflecance-anisotropy spectroscopy of vicinal Si(001)en
dc.type.genreThesisen
thesis.degree.departmentPhysicsen
thesis.degree.disciplinePhysicsen
thesis.degree.grantorThe University of Texas at Austinen
thesis.degree.levelDoctoralen
thesis.degree.nameDoctor of Philosophyen

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